First-order transition in the spin dynamics of geometrically frustrated Yb2Ti2O7.

نویسندگان

  • J A Hodges
  • P Bonville
  • A Forget
  • A Yaouanc
  • P Dalmas de Réotier
  • G André
  • M Rams
  • K Królas
  • C Ritter
  • P C M Gubbens
  • C T Kaiser
  • P J C King
  • C Baines
چکیده

Using neutron diffraction, 170Yb Mössbauer and muon spin relaxation spectroscopies, we have examined the pyrochlore Yb2Ti2O7, where the Yb3+S' = 1/2 ground state has planar anisotropy. Below approximately 0.24 K, the temperature of the known specific-heat lambda transition, there is no long range magnetic order. We show that the transition corresponds to a first-order change in the fluctuation rate of the Yb3+ spins. Above the transition temperature, the rate, in the GHz range, follows a thermal excitation law, whereas below, the rate, in the MHz range, is temperature independent, indicative of a quantum fluctuation regime.

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عنوان ژورنال:
  • Physical review letters

دوره 88 7  شماره 

صفحات  -

تاریخ انتشار 2002